J. Semicond. > 2022, Volume 43 > Issue 5 > 050201, doi: 10.1088/1674-4926/43/5/050201

RESEARCH HIGHLIGHTS

Domain controlling and defect passivation for efficient quasi-2D perovskite LEDs

Dezhong Zhang1, Chuanjiang Qin1, 2, and Liming Ding3,

+ Author Affiliations

 Corresponding author: Chuanjiang Qin, cjqin@ciac.ac.cn; Liming Ding, ding@nanoctr.cn

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[1]
Kim H S, Lee C R, Im J H, et al. Lead iodide perovskite sensitized all-solid-state submicron thin film mesoscopic solar cell with efficiency exceeding 9%. Sci Rep, 2012, 2, 591 doi: 10.1038/srep00591
[2]
Wang N, Cheng L, Ge R, et al. Perovskite light-emitting diodes based on solution-processed self-organized multiple quantum wells. Nat Photonics, 2016, 10, 699 doi: 10.1038/nphoton.2016.185
[3]
Cho H, Jeong S H, Park M H, et al. Overcoming the electroluminescence efficiency limitations of perovskite light-emitting diodes. Science, 2015, 350, 1222 doi: 10.1126/science.aad1818
[4]
Quan L N, Ma D, Zhao Y, et al. Edge stabilization in reduced-dimensional perovskites. Nat Commun, 2020, 11, 170 doi: 10.1038/s41467-019-13944-2
[5]
Jiang Y, Cui M, Li S, et al. Reducing the impact of Auger recombination in quasi-2D perovskite light-emitting diodes. Nat Commun, 2021, 12, 336 doi: 10.1038/s41467-020-20555-9
[6]
Chu Z, Ye Q, Zhao Y, et al. Perovskite light-emitting diodes with external quantum efficiency exceeding 22% via small-molecule passivation. Adv Mater, 2021, 33, 2007169 doi: 10.1002/adma.202007169
[7]
Qin C, Matsushima T, Potscavage W J, et al. Triplet management for efficient perovskite light-emitting diodes. Nat Photonics, 2020, 14, 70 doi: 10.1038/s41566-019-0545-9
[8]
Yuan M, Quan L N, Comin R, et al. Perovskite energy funnels for efficient light-emitting diodes. Nat Nanotechnol, 2016, 11, 872 doi: 10.1038/nnano.2016.110
[9]
Qin C, Sandanayaka A S D, Zhao C, et al. Stable room-temperature continuous-wave lasing in quasi-2D perovskite films. Nature, 2020, 585, 53 doi: 10.1038/s41586-020-2621-1
[10]
Ma D, Lin K, Dong Y, et al. Distribution control enables efficient reduced-dimensional perovskite LEDs. Nature, 2021, 599, 594 doi: 10.1038/s41586-021-03997-z
[11]
Fang Z, Chen W, Shi Y, et al. Dual passivation of perovskite defects for light-emitting diodes with external quantum efficiency exceeding 20%. Adv Funct Mater, 2020, 30, 1909754 doi: 10.1002/adfm.201909754
[12]
Chu Z, Zhao Y, Ma F, et al. Large cation ethylammonium incorporated perovskite for efficient and spectra stable blue light-emitting diodes. Nat Commun, 2020, 11, 4165 doi: 10.1038/s41467-020-17943-6
[13]
Zhang D, Fu Y, Liu C, et al. Domain controlling by compound additive toward highly efficient quasi-2D perovskite light-emitting diodes. Adv Funct Mater, 2021, 31, 2103890 doi: 10.1002/adfm.202103890
[14]
Yantara N, Jamaludin N F, Febriansyah B, et al. Designing the perovskite structural landscape for efficient blue emission. ACS Energy Lett, 2020, 5, 1593 doi: 10.1021/acsenergylett.0c00559
[15]
Kong L, Zhang X, Li Y, et al. Smoothing the energy transfer pathway in quasi-2D perovskite films using methanesulfonate leads to highly efficient light-emitting devices. Nat Commun, 2021, 12, 1246 doi: 10.1038/s41467-021-21522-8
[16]
Akkerman Q A, Rainò G, Kovalenko M V, et al. Genesis, challenges and opportunities for colloidal lead halide perovskite nanocrystals. Nat Mater, 2018, 17, 394 doi: 10.1038/s41563-018-0018-4
[17]
Ye J, Byranvand M M, Martínez C O, et al. Defect passivation in lead-halide perovskite nanocrystals and thin films: toward efficient LEDs and solar cells. Angew Chem Int Ed, 2021, 133, 21804 doi: 10.1002/ange.202102360
[18]
Liu Z, Qiu W, Peng X, et al. Perovskite light-emitting diodes with EQE exceeding 28% through a synergetic dual-additive strategy for defect passivation and nanostructure regulation. Adv Mater, 2021, 33, 2103268 doi: 10.1002/adma.202103268
[19]
Peng X, Yang X, Liu D, et al. Targeted distribution of passivator for polycrystalline perovskite light-emitting diodes with high efficiency. ACS Energy Lett, 2021, 6, 4187 doi: 10.1021/acsenergylett.1c01753
[20]
Zhao C, Wu W, Zhan H, et al. Phosphonate/phosphine oxide dyad additive for efficient perovskite light-emitting diodes. Angew Chem Int Ed, 2022, e202117374 doi: 10.1002/anie.202117374
Fig. 1.  (Color online) (a) Competition between radiative recombination and nonradiative recombination for domains with different n. Reproduced with permission[13], Copyright 2021, Wiley. (b) The strategy to form intermediate domains for emissive quasi-2D perovskite films. Reproduced with permission[14], Copyright 2020, American Chemical Society. (c) Effect of MeS on domain distribution in quasi-2D perovskite films. Reproduced with permission[15], Copyright 2021, Springer Nature. (d) Domain distribution controlling by using TFPPO. Reproduced with permission[10], Copyright 2021, Springer Nature.

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Fig. 2.  (Color online) (a) Degradation mechanisms and edge-stabilization strategy via P=O bonds. Reproduced with permission[4], Copyright 2020, Springer Nature. (b) Schematic illustration of crystal structure change and defect passivation by crown and MPEG-MAA. Reproduced with permission[18], Copyright 2021, Wiley. (c) Passivation mechanism of ionic liquid additive with C=N bond. Reproduced with permission[19], Copyright 2021, American Chemical Society. (d) PE-TPPO-modified PeLED. Reproduced with permission[20], Copyright 2022, Wiley.

DownLoad: Full-Size Img PowerPoint
[1]
Kim H S, Lee C R, Im J H, et al. Lead iodide perovskite sensitized all-solid-state submicron thin film mesoscopic solar cell with efficiency exceeding 9%. Sci Rep, 2012, 2, 591 doi: 10.1038/srep00591
[2]
Wang N, Cheng L, Ge R, et al. Perovskite light-emitting diodes based on solution-processed self-organized multiple quantum wells. Nat Photonics, 2016, 10, 699 doi: 10.1038/nphoton.2016.185
[3]
Cho H, Jeong S H, Park M H, et al. Overcoming the electroluminescence efficiency limitations of perovskite light-emitting diodes. Science, 2015, 350, 1222 doi: 10.1126/science.aad1818
[4]
Quan L N, Ma D, Zhao Y, et al. Edge stabilization in reduced-dimensional perovskites. Nat Commun, 2020, 11, 170 doi: 10.1038/s41467-019-13944-2
[5]
Jiang Y, Cui M, Li S, et al. Reducing the impact of Auger recombination in quasi-2D perovskite light-emitting diodes. Nat Commun, 2021, 12, 336 doi: 10.1038/s41467-020-20555-9
[6]
Chu Z, Ye Q, Zhao Y, et al. Perovskite light-emitting diodes with external quantum efficiency exceeding 22% via small-molecule passivation. Adv Mater, 2021, 33, 2007169 doi: 10.1002/adma.202007169
[7]
Qin C, Matsushima T, Potscavage W J, et al. Triplet management for efficient perovskite light-emitting diodes. Nat Photonics, 2020, 14, 70 doi: 10.1038/s41566-019-0545-9
[8]
Yuan M, Quan L N, Comin R, et al. Perovskite energy funnels for efficient light-emitting diodes. Nat Nanotechnol, 2016, 11, 872 doi: 10.1038/nnano.2016.110
[9]
Qin C, Sandanayaka A S D, Zhao C, et al. Stable room-temperature continuous-wave lasing in quasi-2D perovskite films. Nature, 2020, 585, 53 doi: 10.1038/s41586-020-2621-1
[10]
Ma D, Lin K, Dong Y, et al. Distribution control enables efficient reduced-dimensional perovskite LEDs. Nature, 2021, 599, 594 doi: 10.1038/s41586-021-03997-z
[11]
Fang Z, Chen W, Shi Y, et al. Dual passivation of perovskite defects for light-emitting diodes with external quantum efficiency exceeding 20%. Adv Funct Mater, 2020, 30, 1909754 doi: 10.1002/adfm.201909754
[12]
Chu Z, Zhao Y, Ma F, et al. Large cation ethylammonium incorporated perovskite for efficient and spectra stable blue light-emitting diodes. Nat Commun, 2020, 11, 4165 doi: 10.1038/s41467-020-17943-6
[13]
Zhang D, Fu Y, Liu C, et al. Domain controlling by compound additive toward highly efficient quasi-2D perovskite light-emitting diodes. Adv Funct Mater, 2021, 31, 2103890 doi: 10.1002/adfm.202103890
[14]
Yantara N, Jamaludin N F, Febriansyah B, et al. Designing the perovskite structural landscape for efficient blue emission. ACS Energy Lett, 2020, 5, 1593 doi: 10.1021/acsenergylett.0c00559
[15]
Kong L, Zhang X, Li Y, et al. Smoothing the energy transfer pathway in quasi-2D perovskite films using methanesulfonate leads to highly efficient light-emitting devices. Nat Commun, 2021, 12, 1246 doi: 10.1038/s41467-021-21522-8
[16]
Akkerman Q A, Rainò G, Kovalenko M V, et al. Genesis, challenges and opportunities for colloidal lead halide perovskite nanocrystals. Nat Mater, 2018, 17, 394 doi: 10.1038/s41563-018-0018-4
[17]
Ye J, Byranvand M M, Martínez C O, et al. Defect passivation in lead-halide perovskite nanocrystals and thin films: toward efficient LEDs and solar cells. Angew Chem Int Ed, 2021, 133, 21804 doi: 10.1002/ange.202102360
[18]
Liu Z, Qiu W, Peng X, et al. Perovskite light-emitting diodes with EQE exceeding 28% through a synergetic dual-additive strategy for defect passivation and nanostructure regulation. Adv Mater, 2021, 33, 2103268 doi: 10.1002/adma.202103268
[19]
Peng X, Yang X, Liu D, et al. Targeted distribution of passivator for polycrystalline perovskite light-emitting diodes with high efficiency. ACS Energy Lett, 2021, 6, 4187 doi: 10.1021/acsenergylett.1c01753
[20]
Zhao C, Wu W, Zhan H, et al. Phosphonate/phosphine oxide dyad additive for efficient perovskite light-emitting diodes. Angew Chem Int Ed, 2022, e202117374 doi: 10.1002/anie.202117374

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    Received: 09 March 2022 Revised: Online: Uncorrected proof: 14 March 2022Published: 01 May 2022

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      Article Navigation >  Journal of Semiconductors  > 2022  >  43(5): 050201
      Dezhong Zhang, Chuanjiang Qin, Liming Ding. Domain controlling and defect passivation for efficient quasi-2D perovskite LEDs[J]. Journal of Semiconductors, 2022, 43(5): 050201. doi: 10.1088/1674-4926/43/5/050201 D Z Zhang, C J Qin, L M Ding. Domain controlling and defect passivation for efficient quasi-2D perovskite LEDs[J]. J. Semicond, 2022, 43(5): 050201. doi: 10.1088/1674-4926/43/5/050201Export: BibTex EndNote
      Citation:
      Dezhong Zhang, Chuanjiang Qin, Liming Ding. Domain controlling and defect passivation for efficient quasi-2D perovskite LEDs[J]. Journal of Semiconductors, 2022, 43(5): 050201. doi: 10.1088/1674-4926/43/5/050201

      D Z Zhang, C J Qin, L M Ding. Domain controlling and defect passivation for efficient quasi-2D perovskite LEDs[J]. J. Semicond, 2022, 43(5): 050201. doi: 10.1088/1674-4926/43/5/050201
      Export: BibTex EndNote
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      Domain controlling and defect passivation for efficient quasi-2D perovskite LEDs

      doi: 10.1088/1674-4926/43/5/050201
      • 1.

        State Key Laboratory of Polymer Physics and Chemistry, Changchun Institute of Applied Chemistry, Chinese Academy of Sciences, Changchun 130022, China

      • 2.

        School of Applied Chemistry and Engineering, University of Science and Technology of China, Hefei 230026, China

      • 3.

        Center for Excellence in Nanoscience (CAS), Key Laboratory of Nanosystem and Hierarchical Fabrication (CAS), National Center for Nanoscience and Technology, Beijing 100190, China

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      • Author Bio:

        Dezhong Zhang got his BS in 2013 and PhD in 2019 from Jilin University. Then he joined Chuanjiang Qin Group at Changchun Institute of Applied Chemistry (CAS) as an assistant professor. His research focuses on perovskite solar cells and light-emitting diodes

        Chuanjiang Qin got his PhD from Changchun Institute of Applied Chemistry (CAS) in 2008. Then he worked as a postdoc at Hong Kong Baptist University and National Institute for Materials Science (Japan). Since 2014, he worked with Chihaya Adachi at Center for Organic Photonics and Electronics Research, Kyushu University as a research associate professor. In 2019, he joined Changchun Institute of Applied Chemistry as a full professor. His research focuses on perovskite materials and optoelectronic devices, including perovskite lasers, light-emitting diodes and solar cells

        Liming Ding got his PhD from University of Science and Technology of China (was a joint student at Changchun Institute of Applied Chemistry, CAS). He started his research on OSCs and PLEDs in Olle Ingans Lab in 1998. Later on, he worked at National Center for Polymer Research, Wright-Patterson Air Force Base and Argonne National Lab (USA). He joined Konarka as a Senior Scientist in 2008. In 2010, he joined National Center for Nanoscience and Technology as a full professor. His research focuses on innovative materials and devices. He is RSC Fellow, the nominator for Xplorer Prize, and the Associate Editor for Journal of Semiconductors

      • Corresponding author: cjqin@ciac.ac.cn; ding@nanoctr.cn
      • Received Date: 2022-03-09
        Available Online: 2022-04-27

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