J. Semicond. > 2023, Volume 44 > Issue 3 > 031701, doi: 10.1088/1674-4926/44/3/031701
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REVIEWS

The recent progress of laser-induced graphene based device applications

Liqiang ZhangL, Ziqian ZhouL, Xiaosong Hu and Liaoyong Wen

+ Author Affiliations

 Corresponding author: Xiaosong Hu, huxiaosong@westlake.edu.cn; Liaoyong Wen, wenliaoyong@westlake.edu.cn

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Abstract: Laser writing is a fast and efficient technology that can produce graphene with a high surface area, whereas laser-induced graphene (LIG) has been widely used in both physics and chemical device application. It is necessary to update this important progress because it may provide a clue to consider the current challenges and possible future directions. In this review, the basic principles of LIG fabrication are first briefly described for a detailed understanding of the lasing process. Subsequently, we summarize the physical device applications of LIGs and describe their advantages, including flexible electronics and energy harvesting. Then, chemical device applications are categorized into chemical sensors, supercapacitors, batteries, and electrocatalysis, and a detailed interpretation is provided. Finally, we present our vision of future developments and challenges in this exciting research field.

Key words: laser-induced graphene, flexible electronics, energy harvesting, chemical sensors, supercapacitors, electrocatalysis



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Fig. 1.  (Color online) Representative chemical applications of LIG. Adapted with permission from Ref. [22–24]. Copyright 2016, Wiley-VCH, Copyright 2022, American Chemical Society, Copyright 2020, Elsevier Ltd respectively. Representative physical applications of LIG. Adapted with permission from Ref. [25–27]. Copyright 2020, The Royal Society of Chemistry. Copyright 2021, Hindawi. Copyright 2020, American Chemical Society respectively.

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Fig. 2.  (Color online) (a) Theoretical simulation of LIG synthesis process and the influence of temperature and oxygen on LIG production. Reproduced with permission from Ref. [29]. Copyright 2020, American Chemical Society. (b) Comparison of hydrophilicity of LIG produced in air and N2 atmosphere. Reproduced with permission from Ref. [36]. Copyright 2021, Wiley-VCH.

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Fig. 3.  (Color online) (a) Laser engraved carbonized patterns on Kevlar clothes. Reproduced with permission from Ref. [5]. Copyright 2020, American Chemical Society. (b) Temperature–strain hybrid sensor made by black phosphorus modified LIG. Reproduced with permission from Ref. [43]. Copyright 2020, Wiley-VCH. (c) High permeability stretch sensor based on elastic sponge. Reproduced with permission from Ref. [46]. Copyright 2018, Wiley-VCH.

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Fig. 4.  (Color online) Liquid-solid friction nanogenerator using super-hydrophobic fluorine-doped LIG. Reproduced with permission from Ref. [20]. Copyright 2021, Wiley-VCH.

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Fig. 5.  (Color online) (a) Diagram of a three-electrode sweat UA and Tyr sensors. (b) The different oxidation peak height for the detection of UA and Tyr. (c) Detected signals in the raw sweat samples measured by different electrodes. Reproduced with permission from Ref. [55]. Copyright 2020, Nature Research. (d−g) Schematic illustration, performance, and specificity of the AuNPs/LIG based immunosensor for the detection of Escherichia coli O157:H7. Reproduced with permission from Ref. [58]. Copyright 2020, Elsevier Ltd.

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Fig. 6.  (Color online) (a−c) Schematic diagram of the C−Au−LIG fabrication process and related SEM images. (d) Representative CV curves of different biosensors in standard potassium ferricyanide solution. (e) Redox peak currents of LIG, Au−LIG, and C−Au−LIG after different periods of time in ambient environments. (f) Redox peak currents of LIG, Au−LIG, and C−Au−LIG in continuous usage. Adapted with permission from Ref. [23]. Copyright 2022, American Chemical Society.

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Fig. 7.  (Color online) (a−c) SEM images and the areal specific capacitance of doping LIG. Reproduced with permission from Ref. [75]. Copyright 2022, Elsevier Ltd. (d, e) Electrochemical performance of conductive MOF-derived LIG. Reproduced with permission from Ref. [82]. Copyright 2019, Wiley-VCH. (f) Illustration of customer-designed supercapacitors enabled by laser irradiation. Reproduced with permission from Ref. [83]. Copyright 2019, American Chemical Society. (g) Gaussian beams were transformed into arbitrary geometric target beams by programming phase patterns for the synthesis of different SC. Reproduced with permission from Ref. [84]. Copyright 2020, Nature Research.

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Fig. 8.  (Color online) (a) SEM image, (b) schematic illustration of Li diffusion path, and (c−e) electrochemical performances of a-LIG. Reproduced with permission from Ref. [91]. Copyright 2021, Elsevier Ltd. (f) SEM images of Cu-LiFePO4 full cell after 50 cycles with LI-SiOx coating or not. Reproduced with permission from Ref. [93]. Copyright 2020, Wiley-VCH.

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Fig. 9.  (Color online) (a) Schematic illustration of the synthesis and the electrochemical ORR and antifouling along with antimicrobial properties of S-LIG. Reproduced with permission from Ref. [96]. Copyright 2018, American Chemical Society. (b) Preparation and (c, d) electrochemical performance of LIG-O. Reproduced with permission from Ref. [97]. Copyright 2018, Wiley-VCH. (e) Schematic illustration of formation of MO-LIG from MC-PI film. Reproduced with permission from Ref. [98]. Copyright 2015, American Chemical Society. (f) Photographs and SEM images of different MOF-derived LIG. (g) Comparation of overpotentials for 50 mA/cm2. Reproduced with permission from Ref. [99]. Copyright 2021, Wiley-VCH.

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Fig. 10.  (Color online) (a−c) A full water-splitting device made by laser irradiation followed by electrodeposition and its performance. Reproduced with permission from Ref. [104]. Copyright 2017, American Chemical Society. (d) Preparation and (e) CO2RR performance of the CuSn-LIG catalysts. Reproduced with permission from Ref. [105]. Copyright 2020, American Chemical Society.

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    Received: 02 September 2022 Revised: 19 September 2022 Online: Accepted Manuscript: 29 October 2022Uncorrected proof: 01 November 2022Published: 10 March 2023

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      Article Navigation >  Journal of Semiconductors  > 2023  >  44(3): 031701
      Liqiang Zhang, Ziqian Zhou, Xiaosong Hu, Liaoyong Wen. The recent progress of laser-induced graphene based device applications[J]. Journal of Semiconductors, 2023, 44(3): 031701. doi: 10.1088/1674-4926/44/3/031701 L Q Zhang, Z Q Zhou, X S Hu, L Y Wen. The recent progress of laser-induced graphene based device applications[J]. J. Semicond, 2023, 44(3): 031701. doi: 10.1088/1674-4926/44/3/031701Export: BibTex EndNote
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      Liqiang Zhang, Ziqian Zhou, Xiaosong Hu, Liaoyong Wen. The recent progress of laser-induced graphene based device applications[J]. Journal of Semiconductors, 2023, 44(3): 031701. doi: 10.1088/1674-4926/44/3/031701

      L Q Zhang, Z Q Zhou, X S Hu, L Y Wen. The recent progress of laser-induced graphene based device applications[J]. J. Semicond, 2023, 44(3): 031701. doi: 10.1088/1674-4926/44/3/031701
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      The recent progress of laser-induced graphene based device applications

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      • Key Laboratory of 3D Micro/Nano Fabrication and Characterization of Zhejiang Province, School of Engineering, Westlake University, Hangzhou 310024, China

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        Liqiang Zhang is a postdoctoral fellow at Westlake University, School of Engineering. He received his MS and PhD degrees in Zhejiang University of Technology, School of Material Science and Chemical Engineering in 2015 and 2020 respectively. His main research interests including photoelectrocatalytic reduction of CO2, and electrochemical biosensor

        Ziqian Zhou got her BS and MS degrees from Hunan Agricultural University and South China University of Technology, in 2018 and 2021, respectively. Now she is a PhD student at Westlake University, School of Engineering. Her research focuses on electrocatalysis and biosensor

        Xiaosong Hu is a research associate at the Westlake University, China. He received his PhD degree in Physical Chemistry from Nankai University, China, in 2019. Since 2019, he started his post-doctoral research in School of Engineering, Westlake University. His main research interests include organic/nano catalysis, thermo/electroreduction CO2 and carbon-based single-atoms materials

        Liaoyong Wen obtained his doctoral degree in applied physics from Technical University of Ilmenau, Germany in 2016. He was then promoted as a senior scientist in the IMN MacroNano® (ZIK), Technical University of Ilmenau. Since 2017, he started his post-doctoral research in Institute of Materials Science, University of Connecticut. Dr. Wen joined the School of Engineering in September 2019 as an assistant professor

      • Corresponding author: huxiaosong@westlake.edu.cn; wenliaoyong@westlake.edu.cn
      • Received Date: 2022-09-02
      • Revised Date: 2022-09-19
        • Available Online: 2022-10-29

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