Perovskite/organic tandem solar cells

Jie Sun; Liming Ding

doi:10.1088/1674-4926/44/2/020201

J. Semicond. > 2023, Volume 44 > Issue 2 > 020201, doi: 10.1088/1674-4926/44/2/020201

RESEARCH HIGHLIGHTS

Perovskite/organic tandem solar cells

Jie Sun^{1, 2} and Liming Ding^1,

+ Author Affiliations

Corresponding author: Liming Ding, ding@nanoctr.cn

References

[1]	Zhang L X, Pan X Y, Liu L, et al. Star perovskite materials. J Semicond, 2022, 43, 030203 doi: 10.1088/1674-4926/43/3/030203
[2]	Kim M, Jeong J, Lu H, et al. Conformal quantum dot-SnO₂ layers as electron transporters for efficient perovskite solar cells. Science, 2022, 375, 302 doi: 10.1126/science.abh1885
[3]	Cheng Y H, Ding L M. Perovskite/Si tandem solar cells: Fundamentals, advances, challenges, and novel applications. SusMat, 2021, 1, 324 doi: doi/full/10.1002/sus2.25
[4]	Chen S, Zuo C T, Xu B M, et al. Monolithic perovskite/silicon tandem solar cells offer an efficiency over 29%. J Semicond, 2021, 42, 120203 doi: 10.1088/1674-4926/42/12/120203
[5]	Fang Z M, Zeng Q, Zuo C T, et al. Perovskite-based tandem solar cells. Sci Bull, 2021, 66, 621 doi: 10.1016/j.scib.2020.11.006
[6]	National Renewable Energy Laboratory. Best Research-Cell Efficiencies. 2022
[7]	Zuo C T, Ding L M. Bulk heterojunctions push the photoresponse of perovskite solar cells to 970 nm. J Mater Chem A, 2015, 3, 9063 doi: 10.1039/C4TA04482G
[8]	Chen C C, Bae S H, Chang W H, et al. Perovskite/polymer monolithic hybrid tandem solar cells utilizing a low-temperature, full solution process. Mater Horizons, 2015, 2, 203 doi: 10.1039/C4MH00237G
[9]	Liu Y, Renna L A, Bag M, et al. High efficiency tandem thin-perovskite/polymer solar cells with a graded recombination layer. ACS Appl Mater Interfaces, 2016, 8, 7070 doi: 10.1021/acsami.5b12740
[10]	Brinkmann K O, Becker T, Zimmermann F, et al. Perovskite-organic tandem solar cells with indium oxide interconnect. Nature, 2022, 604, 280 doi: 10.1038/s41586-022-04455-0
[11]	Zeng Q, Liu L, Xiao Z, et al. A two-terminal all-inorganic perovskite/organic tandem solar cell. Sci Bull, 2019, 64, 885 doi: 10.1016/j.scib.2019.05.015
[12]	Xie S, Xia R, Chen Z, et al. Efficient monolithic perovskite/organic tandem solar cells and their efficiency potential. Nano Energy, 2020, 78, 105238 doi: 10.1016/j.nanoen.2020.105238
[13]	Liu L, Xiao Z, Zuo C, et al. Inorganic perovskite/organic tandem solar cells with efficiency over 20%. J Semicond, 2021, 42, 020501 doi: 10.1088/1674-4926/42/2/020501
[14]	Chen W, Li D, Chen X, et al. Surface reconstruction for stable monolithic all-inorganic perovskite/organic tandem solar cells with over 21% efficiency. Adv Funct Mater, 2022, 32, 2109321 doi: 10.1002/adfm.202109321
[15]	Wang P, Li W, Sandberg O J, et al. Tuning of the interconnecting layer for monolithic perovskite/organic tandem solar cells with record efficiency exceeding 21%. Nano Lett, 2021, 21, 7845 doi: 10.1021/acs.nanolett.1c02897
[16]	Chen X, Jia Z Y, Chen Z, et al. Efficient and reproducible monolithic perovskite/organic tandem solar cells with low-loss interconnecting layers. Joule, 2020, 4, 1594 doi: 10.1016/j.joule.2020.06.006
[17]	Xie Y M, Niu T, Yao Q, et al. Understanding the role of interconnecting layer on determining monolithic perovskite/organic tandem device carrier recombination properties. J Energy Chem, 2022, 71, 12 doi: 10.1016/j.jechem.2022.03.019
[18]	Qin S, Lu C, Jia Z, et al. Constructing monolithic perovskite/organic tandem solar cell with efficiency of 22.0% via reduced open-circuit voltage loss and broadened absorption spectra. Adv Mater, 2022, 34, 2108829 doi: 10.1002/adma.202108829
[19]	Chen W, Zhu Y, Xiu J, et al. Monolithic perovskite/organic tandem solar cells with 23.6% efficiency enabled by reduced voltage losses and optimized interconnecting layer. Nat Energy, 2022, 7, 229 doi: 10.1038/s41560-021-00966-8
[20]	Li Z, Wu S F, Zhang J, et al. Hybrid perovskite-organic flexible tandem solar cell enabling highly efficient electrocatalysis overall water splitting. Adv Energy Mater, 2020, 10, 2000361 doi: 10.1002/aenm.202000361
[21]	Xie Y M, Yao Q, Zeng Z, et al. Homogeneous grain boundary passivation in wide-bandgap perovskite films enables fabrication of monolithic perovskite/organic tandem solar cells with over 21% efficiency. Adv Funct Mater, 2022, 32, 2112126 doi: 10.1002/adfm.202112126

Fig. 1. (Color online) The structure for perovskite-organic tandem solar cells.

DownLoad: Full-Size Img PowerPoint

Fig. 2. (Color online) The PCE advance for perovskite-organic tandem solar cells.

DownLoad: Full-Size Img PowerPoint

Table 1. Performance data for perovskite-organic tandem solar cells. (* indicates the certified PCE)

Front cell	ICL	Rear cell	V_oc (V)	J_sc (mA/cm²)	FF (%)	PCE (%)	Ref.
ITO/PEDOT:PSS/PBSeDTEG8:PC₆₁BM/PFN/TiO₂	PEDOT:PSS PH500/PEDOT:PSS 4083	CH₃NH₃PbI₃/PC₆₁BM/PFN/Al	1.52	10.05	67.0	10.23	[8]
ITO/PEDOT:PSS/CH₃NH₃PbI₃/PC₆₁BM	C₆₀-SB/Ag/MoO₃	PCE-10:PC₇₁BM/C₆₀-N/Ag	1.62	12.90	75.0	16.00	[9]
ITO/SnO₂/CsPbI₂Br/PTAA	MoO₃/Au/ZnO	PTB7-Th:CO_i8DFIC:PC₇₁BM/ MoO₃/Ag	1.71	11.98	73.4	15.04	[11]
ITO/PTAA/Cs_0.1(FA_0.6MA_0.4)_0.9Pb(I_0.6Br_0.4)₃/ PC₆₁BM/BCP	Ag/PEDOT:PSS	PBDB-T:SN6IC-4F/C60-bis/ BCP/Ag	1.85	11.52	71.0	15.13	[20]
ITO/ZnO/SnO₂/CsPbI₂Br/PDCBT	MoO₃/Ag/ZnO	PM6:Y6/MoO₃/Ag	1.95	12.46	75.6	18.38	[12]
ITO/NiO_x/FA_0.8MA_0.02Cs_0.18PbI_1.8Br_1.2/C₆₀	BCP/Ag/MoO_x	PBDBT-2F:Y6:PC₇₁BM/TPBi/Ag	1.90	13.05	83.1	19.54*	[16]
ITO/SnO₂/ZnO/CsPbI₂Br	PTAA/MoO₃/Au/ZnO	D18:Y6/MoO₃/Ag	2.05	13.07	25.3	20.18	[13]
ITO/SnO₂/CsPbI_1.8Br_1.2/TACl	PBDB-T/MoO₃/Au/ ZnO/PFN	PM6:Y6/MoO₃/Al	2.05	13.36	76.8	21.04	[14]
ITO/ZnO/CsPbI₂Br/polyTPD	MoO₃/Ag/PFN-Br	PM6:Y6-BO/MoO₃/Ag	1.96	13.30	80.8	21.10	[15]
ITO/Poly-TPD/(MAPbI₂Br + Pb(SCN)₂)	PCBM/BCP/Au/MoO₃	PM6:Y6/PFN-Br/Ag	1.94	13.12	78.7	20.03	[17]
ITO/poly-TPD/(MA_0.9FA_0.1PbI₂Br + Pb(SCN)₂)	PCBM/BCP/Au/MoO₃	PM6:CH1007/PFN-Br/Ag	1.96	13.80	78.4	21.2	[21]
ITO/2PACz/FA_0.6MA_0.4Pb(I_0.6Br_0.4)₃	C₆₀/BCP/Ag/MoO_x	PTB7-Th:BTPV-4Cl-eC9/ PDINN/Ag	1.88	15.70	74.6	22.00	[18]
ITO/PTAA/FA_0.8Cs_0.2Pb(I_0.5Br_0.5)₃/PEAI/ PC₆₁BM/AZO-NP	SnO_x/InO_x/MoO_x	PM6:Y6:PC₆₁BM/C₆₀/BCP/Ag	2.15	14.00	80.0	23.10*	[10]
ITO/NiO_x/BPA/Cs_0.25FA_0.75Pb(I_0.6Br_0.4)₃	C₆₀/BCP/CRL/MoO_x	PM6:Y6/PNDIT-F3N/Ag	2.05	14.83	77.2	22.94*	[19]

DownLoad: CSV

[1]	Zhang L X, Pan X Y, Liu L, et al. Star perovskite materials. J Semicond, 2022, 43, 030203 doi: 10.1088/1674-4926/43/3/030203
[2]	Kim M, Jeong J, Lu H, et al. Conformal quantum dot-SnO₂ layers as electron transporters for efficient perovskite solar cells. Science, 2022, 375, 302 doi: 10.1126/science.abh1885
[3]	Cheng Y H, Ding L M. Perovskite/Si tandem solar cells: Fundamentals, advances, challenges, and novel applications. SusMat, 2021, 1, 324 doi: doi/full/10.1002/sus2.25
[4]	Chen S, Zuo C T, Xu B M, et al. Monolithic perovskite/silicon tandem solar cells offer an efficiency over 29%. J Semicond, 2021, 42, 120203 doi: 10.1088/1674-4926/42/12/120203
[5]	Fang Z M, Zeng Q, Zuo C T, et al. Perovskite-based tandem solar cells. Sci Bull, 2021, 66, 621 doi: 10.1016/j.scib.2020.11.006
[6]	National Renewable Energy Laboratory. Best Research-Cell Efficiencies. 2022
[7]	Zuo C T, Ding L M. Bulk heterojunctions push the photoresponse of perovskite solar cells to 970 nm. J Mater Chem A, 2015, 3, 9063 doi: 10.1039/C4TA04482G
[8]	Chen C C, Bae S H, Chang W H, et al. Perovskite/polymer monolithic hybrid tandem solar cells utilizing a low-temperature, full solution process. Mater Horizons, 2015, 2, 203 doi: 10.1039/C4MH00237G
[9]	Liu Y, Renna L A, Bag M, et al. High efficiency tandem thin-perovskite/polymer solar cells with a graded recombination layer. ACS Appl Mater Interfaces, 2016, 8, 7070 doi: 10.1021/acsami.5b12740
[10]	Brinkmann K O, Becker T, Zimmermann F, et al. Perovskite-organic tandem solar cells with indium oxide interconnect. Nature, 2022, 604, 280 doi: 10.1038/s41586-022-04455-0
[11]	Zeng Q, Liu L, Xiao Z, et al. A two-terminal all-inorganic perovskite/organic tandem solar cell. Sci Bull, 2019, 64, 885 doi: 10.1016/j.scib.2019.05.015
[12]	Xie S, Xia R, Chen Z, et al. Efficient monolithic perovskite/organic tandem solar cells and their efficiency potential. Nano Energy, 2020, 78, 105238 doi: 10.1016/j.nanoen.2020.105238
[13]	Liu L, Xiao Z, Zuo C, et al. Inorganic perovskite/organic tandem solar cells with efficiency over 20%. J Semicond, 2021, 42, 020501 doi: 10.1088/1674-4926/42/2/020501
[14]	Chen W, Li D, Chen X, et al. Surface reconstruction for stable monolithic all-inorganic perovskite/organic tandem solar cells with over 21% efficiency. Adv Funct Mater, 2022, 32, 2109321 doi: 10.1002/adfm.202109321
[15]	Wang P, Li W, Sandberg O J, et al. Tuning of the interconnecting layer for monolithic perovskite/organic tandem solar cells with record efficiency exceeding 21%. Nano Lett, 2021, 21, 7845 doi: 10.1021/acs.nanolett.1c02897
[16]	Chen X, Jia Z Y, Chen Z, et al. Efficient and reproducible monolithic perovskite/organic tandem solar cells with low-loss interconnecting layers. Joule, 2020, 4, 1594 doi: 10.1016/j.joule.2020.06.006
[17]	Xie Y M, Niu T, Yao Q, et al. Understanding the role of interconnecting layer on determining monolithic perovskite/organic tandem device carrier recombination properties. J Energy Chem, 2022, 71, 12 doi: 10.1016/j.jechem.2022.03.019
[18]	Qin S, Lu C, Jia Z, et al. Constructing monolithic perovskite/organic tandem solar cell with efficiency of 22.0% via reduced open-circuit voltage loss and broadened absorption spectra. Adv Mater, 2022, 34, 2108829 doi: 10.1002/adma.202108829
[19]	Chen W, Zhu Y, Xiu J, et al. Monolithic perovskite/organic tandem solar cells with 23.6% efficiency enabled by reduced voltage losses and optimized interconnecting layer. Nat Energy, 2022, 7, 229 doi: 10.1038/s41560-021-00966-8
[20]	Li Z, Wu S F, Zhang J, et al. Hybrid perovskite-organic flexible tandem solar cell enabling highly efficient electrocatalysis overall water splitting. Adv Energy Mater, 2020, 10, 2000361 doi: 10.1002/aenm.202000361
[21]	Xie Y M, Yao Q, Zeng Z, et al. Homogeneous grain boundary passivation in wide-bandgap perovskite films enables fabrication of monolithic perovskite/organic tandem solar cells with over 21% efficiency. Adv Funct Mater, 2022, 32, 2112126 doi: 10.1002/adfm.202112126