J. Semicond. > 2024, Volume 45 > Issue 2 > 020202

RESEARCH HIGHLIGHTS

Engineering fibrillar morphology for highly efficient organic solar cells

Chengcheng Xie1, Bin Zhang1, Menglan Lv1, and Liming Ding2,

+ Author Affiliations

 Corresponding author: Menglan Lv, mllv@gzu.edu.cn; Liming Ding, ding@nanoctr.cn

DOI: 10.1088/1674-4926/45/2/020202

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[1]
Wei Y N, Chen Z H, Lu G Y, et al. Binary organic solar cells breaking 19% via manipulating the vertical component distribution. Adv Mater, 2022, 34(33), 2204718 doi: 10.1002/adma.202204718
[2]
Zhou M W, Liao C T, Duan Y W, et al. 19.10% efficiency and 80.5% fill factor layer-by-layer organic solar cells realized by 4-bis(2-thienyl)Pyrrole-2, 5-dione based polymer additives for inducing vertical segregation morphology. Adv Mater, 2023, 35(6), 2208279 doi: 10.1002/adma.202208279
[3]
Chen T Y, Li S X, Li Y K, et al. Compromising charge generation and recombination of organic photovoltaics with mixed diluent strategy for certified 19.4% efficiency. Adv Mater, 2023, 35(21), 2300400 doi: 10.1002/adma.202300400
[4]
Ma R J, Yan C Q, Yu J S, et al. High-efficiency ternary organic solar cells with a good figure-of-merit enabled by two low-cost donor polymers. ACS Energy Lett, 2022, 7(8), 2547 doi: 10.1021/acsenergylett.2c01364
[5]
Zhang G C, Lin F R, Qi F, et al. Renewed prospects for organic photovoltaics. Chem Rev, 2022, 122(18), 14180 doi: 10.1021/acs.chemrev.1c00955
[6]
Cao J M, Yi L F, Ding L M. The origin and evolution of Y6 structure. J Semicond, 2022, 43(3), 030202 doi: 10.1088/1674-4926/43/3/030202
[7]
Liu Q S, Jiang Y F, Jin K, et al. 18% efficiency organic solar cells. Sci Bull (Beijing), 2020, 65(4), 272 doi: 10.1016/j.scib.2020.01.001
[8]
Cao J M, Nie G G, Zhang L X, et al. Star polymer donors. J Semicond, 2022, 43(7), 070201 doi: 10.1088/1674-4926/43/7/070201
[9]
Meng X Y, Jin K, Xiao Z, et al. Side chain engineering on D18 polymers yields 18.74% power conversion efficiency. J Semicond, 2021, 42(10), 100501 doi: 10.1088/1674-4926/42/10/100501
[10]
Jin K, Xiao Z, Ding L M. D18, an eximious solar polymer! J Semicond, 2021, 42(1), 010502 doi: 10.1088/1674-4926/42/1/010502
[11]
Jin K, Xiao Z, Ding L M. 18.69% PCE from organic solar cells. J Semicond, 2021, 42(6), 060502 doi: 10.1088/1674-4926/42/6/060502
[12]
Qin J Q, Zhang L X, Zuo C T, et al. A chlorinated copolymer donor demonstrates a 18.13% power conversion efficiency. J Semicond, 2021, 42(1), 010501 doi: 10.1088/1674-4926/42/1/010501
[13]
Zhou J, Li D H, Wang L, et al. Bicontinuous donor and acceptor fibril networks enable 19.2% efficiency pseudo-bulk heterojunction organic solar cells. Interdiscip Mater, 2023, 2(6), 866 doi: 10.1002/idm2.12129
[14]
Su Y L, Zhang L, Ding Z C, et al. Carrier generation engineering toward 18% efficiency organic solar cells by controlling film microstructure. Adv Energy Mater, 2022, 12(19), 2103940 doi: 10.1002/aenm.202103940
[15]
Zhu L, Zhang M, Xu J Q, et al. Single-junction organic solar cells with over 19% efficiency enabled by a refined double-fibril network morphology. Nat Mater, 2022, 21(6), 656 doi: 10.1038/s41563-022-01244-y
[16]
Li D H, Deng N, Fu Y W, et al. Fibrillization of non-fullerene acceptors enables 19% efficiency pseudo-bulk heterojunction organic solar cells. Adv Mater, 2023, 35(6), 2208211 doi: 10.1002/adma.202208211
[17]
Bi P Q, Wang J Q, Cui Y, et al. Enhancing photon utilization efficiency for high-performance organic photovoltaic cells via regulating phase-transition kinetics. Adv Mater, 2023, 35(16), 2210865 doi: 10.1002/adma.202210865
[18]
Wang J Q, Wang Y F, Bi P Q, et al. Binary organic solar cells with 19.2% efficiency enabled by solid additive. Adv Mater, 2023, 35(25), e2301583 doi: 10.1002/adma.202301583
[19]
Ma L J, Cui Y, Zhang J Q, et al. High-efficiency and mechanically robust all-polymer organic photovoltaic cells enabled by optimized fibril network morphology. Adv Mater, 2023, 35(9), 2208926 doi: 10.1002/adma.202208926
[20]
Zeng R, Zhu L, Zhang M, et al. All-polymer organic solar cells with nano-to-micron hierarchical morphology and large light receiving angle. Nat Commun, 2023, 14(1), 4148 doi: 10.1038/s41467-023-39832-4
Fig. 1.  (Color online) Chemical structures for the star donors and acceptors.

[1]
Wei Y N, Chen Z H, Lu G Y, et al. Binary organic solar cells breaking 19% via manipulating the vertical component distribution. Adv Mater, 2022, 34(33), 2204718 doi: 10.1002/adma.202204718
[2]
Zhou M W, Liao C T, Duan Y W, et al. 19.10% efficiency and 80.5% fill factor layer-by-layer organic solar cells realized by 4-bis(2-thienyl)Pyrrole-2, 5-dione based polymer additives for inducing vertical segregation morphology. Adv Mater, 2023, 35(6), 2208279 doi: 10.1002/adma.202208279
[3]
Chen T Y, Li S X, Li Y K, et al. Compromising charge generation and recombination of organic photovoltaics with mixed diluent strategy for certified 19.4% efficiency. Adv Mater, 2023, 35(21), 2300400 doi: 10.1002/adma.202300400
[4]
Ma R J, Yan C Q, Yu J S, et al. High-efficiency ternary organic solar cells with a good figure-of-merit enabled by two low-cost donor polymers. ACS Energy Lett, 2022, 7(8), 2547 doi: 10.1021/acsenergylett.2c01364
[5]
Zhang G C, Lin F R, Qi F, et al. Renewed prospects for organic photovoltaics. Chem Rev, 2022, 122(18), 14180 doi: 10.1021/acs.chemrev.1c00955
[6]
Cao J M, Yi L F, Ding L M. The origin and evolution of Y6 structure. J Semicond, 2022, 43(3), 030202 doi: 10.1088/1674-4926/43/3/030202
[7]
Liu Q S, Jiang Y F, Jin K, et al. 18% efficiency organic solar cells. Sci Bull (Beijing), 2020, 65(4), 272 doi: 10.1016/j.scib.2020.01.001
[8]
Cao J M, Nie G G, Zhang L X, et al. Star polymer donors. J Semicond, 2022, 43(7), 070201 doi: 10.1088/1674-4926/43/7/070201
[9]
Meng X Y, Jin K, Xiao Z, et al. Side chain engineering on D18 polymers yields 18.74% power conversion efficiency. J Semicond, 2021, 42(10), 100501 doi: 10.1088/1674-4926/42/10/100501
[10]
Jin K, Xiao Z, Ding L M. D18, an eximious solar polymer! J Semicond, 2021, 42(1), 010502 doi: 10.1088/1674-4926/42/1/010502
[11]
Jin K, Xiao Z, Ding L M. 18.69% PCE from organic solar cells. J Semicond, 2021, 42(6), 060502 doi: 10.1088/1674-4926/42/6/060502
[12]
Qin J Q, Zhang L X, Zuo C T, et al. A chlorinated copolymer donor demonstrates a 18.13% power conversion efficiency. J Semicond, 2021, 42(1), 010501 doi: 10.1088/1674-4926/42/1/010501
[13]
Zhou J, Li D H, Wang L, et al. Bicontinuous donor and acceptor fibril networks enable 19.2% efficiency pseudo-bulk heterojunction organic solar cells. Interdiscip Mater, 2023, 2(6), 866 doi: 10.1002/idm2.12129
[14]
Su Y L, Zhang L, Ding Z C, et al. Carrier generation engineering toward 18% efficiency organic solar cells by controlling film microstructure. Adv Energy Mater, 2022, 12(19), 2103940 doi: 10.1002/aenm.202103940
[15]
Zhu L, Zhang M, Xu J Q, et al. Single-junction organic solar cells with over 19% efficiency enabled by a refined double-fibril network morphology. Nat Mater, 2022, 21(6), 656 doi: 10.1038/s41563-022-01244-y
[16]
Li D H, Deng N, Fu Y W, et al. Fibrillization of non-fullerene acceptors enables 19% efficiency pseudo-bulk heterojunction organic solar cells. Adv Mater, 2023, 35(6), 2208211 doi: 10.1002/adma.202208211
[17]
Bi P Q, Wang J Q, Cui Y, et al. Enhancing photon utilization efficiency for high-performance organic photovoltaic cells via regulating phase-transition kinetics. Adv Mater, 2023, 35(16), 2210865 doi: 10.1002/adma.202210865
[18]
Wang J Q, Wang Y F, Bi P Q, et al. Binary organic solar cells with 19.2% efficiency enabled by solid additive. Adv Mater, 2023, 35(25), e2301583 doi: 10.1002/adma.202301583
[19]
Ma L J, Cui Y, Zhang J Q, et al. High-efficiency and mechanically robust all-polymer organic photovoltaic cells enabled by optimized fibril network morphology. Adv Mater, 2023, 35(9), 2208926 doi: 10.1002/adma.202208926
[20]
Zeng R, Zhu L, Zhang M, et al. All-polymer organic solar cells with nano-to-micron hierarchical morphology and large light receiving angle. Nat Commun, 2023, 14(1), 4148 doi: 10.1038/s41467-023-39832-4
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    Received: 15 January 2024 Revised: Online: Accepted Manuscript: 18 January 2024Uncorrected proof: 18 January 2024Published: 10 February 2024

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      Chengcheng Xie, Bin Zhang, Menglan Lv, Liming Ding. Engineering fibrillar morphology for highly efficient organic solar cells[J]. Journal of Semiconductors, 2024, 45(2): 020202. doi: 10.1088/1674-4926/45/2/020202 ****Chengcheng Xie, Bin Zhang, Menglan Lv, Liming Ding. 2024: Engineering fibrillar morphology for highly efficient organic solar cells. Journal of Semiconductors, 45(2): 020202. doi: 10.1088/1674-4926/45/2/020202
      Citation:
      Chengcheng Xie, Bin Zhang, Menglan Lv, Liming Ding. Engineering fibrillar morphology for highly efficient organic solar cells[J]. Journal of Semiconductors, 2024, 45(2): 020202. doi: 10.1088/1674-4926/45/2/020202 ****
      Chengcheng Xie, Bin Zhang, Menglan Lv, Liming Ding. 2024: Engineering fibrillar morphology for highly efficient organic solar cells. Journal of Semiconductors, 45(2): 020202. doi: 10.1088/1674-4926/45/2/020202

      Engineering fibrillar morphology for highly efficient organic solar cells

      DOI: 10.1088/1674-4926/45/2/020202
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      • Chengcheng Xie received his PhD from Beijing University of Chemical Technology in 2023. Then he joined Guizhou University as an associate professor. His research focuses on organic solar cells
      • Bin Zhang got his BS from East China University of Technology in 2005. Then, he got his MS and PhD degrees from South China University of Technology (SCUT) in 2008 and 2012, respectively. From 2013 to 2017, he did postdoctoral research in SCUT and Shenzhen University. In 2018, he joined Changzhou University and was appointed as an associate professor. Now, he is a professor in School of Chemistry and Chemical Engineering, Guizhou University. His research focuses on organic semiconductors and perovskite solar cells
      • Menglan Lv received her PhD from Chengdu Institute of Organic Chemistry, Chinese Academy of Sciences in 2014. She is currently a professor at Guizhou University. Her research focuses on organic solar cells
      • Liming Ding got his PhD from University of Science and Technology of China (was a joint student at Changchun Institute of Applied Chemistry, CAS). He started his research on OSCs and PLEDs in Olle Inganäs Lab in 1998. Later on, he worked at National Center for Polymer Research, Wright-Patterson Air Force Base and Argonne National Lab (USA). He joined Konarka as a Senior Scientist in 2008. In 2010, he joined National Center for Nanoscience and Technology as a full professor. His research focuses on innovative materials and devices. He is RSC Fellow, and the Associate Editors for Journal of Semiconductors and DeCarbon
      • Corresponding author: mllv@gzu.edu.cnding@nanoctr.cn
      • Received Date: 2024-01-15
        Available Online: 2024-01-18

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