J. Semicond. > 2021, Volume 42 > Issue 2 > 020501, doi: 10.1088/1674-4926/42/2/020501
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Inorganic perovskite/organic tandem solar cells with efficiency over 20%

Ling Liu1, 2, Zuo Xiao1, Chuantian Zuo1, and Liming Ding1, 2,

+ Author Affiliations

 Corresponding author: Chuantian Zuo, zuocht@nanoctr.cn; Liming Ding, ding@nanoctr.cn

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[1]
Xiao Z, Yang S, Yang Z, et al. Carbon-oxygen-bridged ladder-type building blocks for highly efficient nonfullerene acceptors. Adv Mater, 2019, 31, e1804790 doi: 10.1002/adma.201804790
[2]
Jia X, Zuo C, Tao S, et al. CsPb(IxBr1−x)3 solar cells. Sci Bull, 2019, 64, 1532 doi: 10.1016/j.scib.2019.08.017
[3]
Chen W, Chen H, Xu G, et al. Precise control of crystal growth for highly efficient CsPbI2Br perovskite solar cells. Joule, 2019, 3, 191 doi: 10.1016/j.joule.2018.10.011
[4]
He J, Liu J, Hou Y, et al. Surface chelation of cesium halide perovskite by dithiocarbamate for efficient and stable solar cells. Nat Commun, 2020, 11, 4237 doi: 10.1038/s41467-020-18015-5
[5]
Zeng Q, Liu L, Xiao Z, et al. A two-terminal all-inorganic perovskite/organic tandem solar cell. Sci Bull, 2019, 64, 885 doi: 10.1016/j.scib.2019.05.015
[6]
Xu J, Boyd C C, Yu Z J, et al. Triple-halide wide-bandgap perovskites with suppressed phase segregation for efficient tandems. Science, 2020, 367, 1097 doi: 10.1126/science.aaz5074
[7]
Al-Ashouri A, Magomedov A, Roß M, et al. Conformal monolayer contacts with lossless interfaces for perovskite single junction and monolithic tandem solar cells. Energy Environ Sci, 2019, 12, 3356 doi: 10.1039/C9EE02268F
[8]
Xiao K, Lin R, Han Q, et al. All-perovskite tandem solar cells with 24.2% certified efficiency and area over 1 cm2 using surface-anchoring zwitterionic antioxidant. Nat Energy, 2020, 5, 870 doi: 10.1038/s41560-020-00705-5
[9]
Chen X, Jia Z, Chen Z, et al. Efficient and reproducible monolithic perovskite/organic tandem solar cells with low-loss interconnecting layers. Joule, 2020, 4, 1594 doi: 10.1016/j.joule.2020.06.006
[10]
Fang Z, Zeng Q, Zuo C, et al. Perovskite-based tandem solar cells. Sci Bull, 2020 doi: 10.1016/j.scib.2020.11.006
[11]
Xie S, Xia R, Chen Z, et al. Efficient monolithic perovskite/organic tandem solar cells and their efficiency potential. Nano Energy, 2020, 78, 105238 doi: 10.1016/j.nanoen.2020.105238
[12]
Liu Q, Jiang Y, Jin K, et al. 18% efficiency organic solar cells. Sci Bull, 2020, 65, 272 doi: 10.1016/j.scib.2020.01.001
[13]
Jin K, Xiao Z, Ding L. D18, an eximious solar polymer!. J Semicond, 2021, 42, 010502 doi: 0.1088/1674-4926/42/1/010502
[14]
Yuan J, Zhang Y, Zhou L, et al. Single-junction organic solar cell with over 15% efficiency using fused-ring acceptor with electron-deficient core. Joule, 2019, 3, 1140 doi: 10.1016/j.joule.2019.01.004
[15]
Li Y, Lin J D, Liu X, et al. Near-infrared ternary tandem solar cells. Adv Mater, 2018, 30, e1804416 doi: 10.1002/adma.201804416
[16]
Meng L, Yi Y Q, Wan X, et al. A tandem organic solar cell with PCE of 14.52% employing subcells with the same polymer donor and two absorption complementary acceptors. Adv Mater, 2019, 31, e1804723 doi: 10.1002/adma.201804723
[17]
Liu G, Jia J, Zhang K, et al. 15% efficiency tandem organic solar cell based on a novel highly efficient wide-bandgap nonfullerene acceptor with low energy loss. Adv Energy Mater, 2019, 9, 1803657 doi: 10.1002/aenm.201803657
[18]
Ramírez Quiroz C O, Spyropoulos G D, Salvador M, et al. Interface molecular engineering for laminated monolithic perovskite/silicon tandem solar cells with 80.4% fill factor. Adv Funct Mater, 2019, 29, 1901476 doi: 10.1002/adfm.201901476
[19]
Li N, Brabec C J. Air-processed polymer tandem solar cells with power conversion efficiency exceeding 10%. Energy Environ Sci, 2015, 8, 2902 doi: 10.1039/C5EE02145F
[20]
Li W, Furlan A, Hendriks K H, et al. Efficient tandem and triple-junction polymer solar cells. J Am Chem Soc, 2013, 135, 5529 doi: 10.1021/ja401434x
[21]
Cheng P, Liu Y, Chang S, et al. Efficient tandem organic photovoltaics with tunable rear sub-cells. Joule, 2019, 3, 432 doi: 10.1016/j.joule.2018.11.011
[22]
Seo J, Moon Y, Lee S, et al. High efficiency tandem polymer solar cells with MoO3/Ni/ZnO:PEOz hybrid interconnection layers. Nanoscale Horiz, 2019, 4, 1221 doi: 10.1039/C9NH00209J
[23]
Li M, Gao K, Wan X, et al. Solution-processed organic tandem solar cells with power conversion efficiencies > 12%. Nat Photonics, 2016, 11, 85 doi: 10.1038/nphoton.2016.240
[24]
Meng L, Zhang Y, Wan X, et al. Organic and solution-processed tandem solar cells with 17.3% efficiency. Science, 2018, 361, 1094 doi: 10.1126/science.aat2612
[25]
Cui Y, Yao H, Gao B, et al. Fine-tuned photoactive and interconnection layers for achieving over 13% efficiency in a fullerene-free tandem organic solar cell. J Am Chem Soc, 2017, 139, 7302 doi: 10.1021/jacs.7b01493
[26]
Aqoma H, Imran I F, Wibowo F T A, et al. High-efficiency solution-processed two-terminal hybrid tandem solar cells using spectrally matched inorganic and organic photoactive materials. Adv Energy Mater, 2020, 10, 2001188 doi: 10.1002/aenm.202001188
[27]
Lang K, Guo Q, He Z, et al. High performance tandem solar cells with inorganic perovskite and organic conjugated molecules to realize complementary absorption. J Phys Chem Lett, 2020, 11, 9596 doi: 10.1021/acs.jpclett.0c02794
Fig. 1.  (Color online) (a) Structures for D18 and Y6. (b) Absorption spectra for CsPbI2Br and D18:Y6 (1 : 1.6) films. (c) The cross-section SEM image for the tandem cell. (d) J–V curve for the best tandem cell. (e) EQE spectra for the front subcell and rear subcell. (f) Summary of the Voc and PCE for the tandem cell in this work and the reported organic/organic and inorganic/organic tandem cells.

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[1]
Xiao Z, Yang S, Yang Z, et al. Carbon-oxygen-bridged ladder-type building blocks for highly efficient nonfullerene acceptors. Adv Mater, 2019, 31, e1804790 doi: 10.1002/adma.201804790
[2]
Jia X, Zuo C, Tao S, et al. CsPb(IxBr1−x)3 solar cells. Sci Bull, 2019, 64, 1532 doi: 10.1016/j.scib.2019.08.017
[3]
Chen W, Chen H, Xu G, et al. Precise control of crystal growth for highly efficient CsPbI2Br perovskite solar cells. Joule, 2019, 3, 191 doi: 10.1016/j.joule.2018.10.011
[4]
He J, Liu J, Hou Y, et al. Surface chelation of cesium halide perovskite by dithiocarbamate for efficient and stable solar cells. Nat Commun, 2020, 11, 4237 doi: 10.1038/s41467-020-18015-5
[5]
Zeng Q, Liu L, Xiao Z, et al. A two-terminal all-inorganic perovskite/organic tandem solar cell. Sci Bull, 2019, 64, 885 doi: 10.1016/j.scib.2019.05.015
[6]
Xu J, Boyd C C, Yu Z J, et al. Triple-halide wide-bandgap perovskites with suppressed phase segregation for efficient tandems. Science, 2020, 367, 1097 doi: 10.1126/science.aaz5074
[7]
Al-Ashouri A, Magomedov A, Roß M, et al. Conformal monolayer contacts with lossless interfaces for perovskite single junction and monolithic tandem solar cells. Energy Environ Sci, 2019, 12, 3356 doi: 10.1039/C9EE02268F
[8]
Xiao K, Lin R, Han Q, et al. All-perovskite tandem solar cells with 24.2% certified efficiency and area over 1 cm2 using surface-anchoring zwitterionic antioxidant. Nat Energy, 2020, 5, 870 doi: 10.1038/s41560-020-00705-5
[9]
Chen X, Jia Z, Chen Z, et al. Efficient and reproducible monolithic perovskite/organic tandem solar cells with low-loss interconnecting layers. Joule, 2020, 4, 1594 doi: 10.1016/j.joule.2020.06.006
[10]
Fang Z, Zeng Q, Zuo C, et al. Perovskite-based tandem solar cells. Sci Bull, 2020 doi: 10.1016/j.scib.2020.11.006
[11]
Xie S, Xia R, Chen Z, et al. Efficient monolithic perovskite/organic tandem solar cells and their efficiency potential. Nano Energy, 2020, 78, 105238 doi: 10.1016/j.nanoen.2020.105238
[12]
Liu Q, Jiang Y, Jin K, et al. 18% efficiency organic solar cells. Sci Bull, 2020, 65, 272 doi: 10.1016/j.scib.2020.01.001
[13]
Jin K, Xiao Z, Ding L. D18, an eximious solar polymer!. J Semicond, 2021, 42, 010502 doi: 0.1088/1674-4926/42/1/010502
[14]
Yuan J, Zhang Y, Zhou L, et al. Single-junction organic solar cell with over 15% efficiency using fused-ring acceptor with electron-deficient core. Joule, 2019, 3, 1140 doi: 10.1016/j.joule.2019.01.004
[15]
Li Y, Lin J D, Liu X, et al. Near-infrared ternary tandem solar cells. Adv Mater, 2018, 30, e1804416 doi: 10.1002/adma.201804416
[16]
Meng L, Yi Y Q, Wan X, et al. A tandem organic solar cell with PCE of 14.52% employing subcells with the same polymer donor and two absorption complementary acceptors. Adv Mater, 2019, 31, e1804723 doi: 10.1002/adma.201804723
[17]
Liu G, Jia J, Zhang K, et al. 15% efficiency tandem organic solar cell based on a novel highly efficient wide-bandgap nonfullerene acceptor with low energy loss. Adv Energy Mater, 2019, 9, 1803657 doi: 10.1002/aenm.201803657
[18]
Ramírez Quiroz C O, Spyropoulos G D, Salvador M, et al. Interface molecular engineering for laminated monolithic perovskite/silicon tandem solar cells with 80.4% fill factor. Adv Funct Mater, 2019, 29, 1901476 doi: 10.1002/adfm.201901476
[19]
Li N, Brabec C J. Air-processed polymer tandem solar cells with power conversion efficiency exceeding 10%. Energy Environ Sci, 2015, 8, 2902 doi: 10.1039/C5EE02145F
[20]
Li W, Furlan A, Hendriks K H, et al. Efficient tandem and triple-junction polymer solar cells. J Am Chem Soc, 2013, 135, 5529 doi: 10.1021/ja401434x
[21]
Cheng P, Liu Y, Chang S, et al. Efficient tandem organic photovoltaics with tunable rear sub-cells. Joule, 2019, 3, 432 doi: 10.1016/j.joule.2018.11.011
[22]
Seo J, Moon Y, Lee S, et al. High efficiency tandem polymer solar cells with MoO3/Ni/ZnO:PEOz hybrid interconnection layers. Nanoscale Horiz, 2019, 4, 1221 doi: 10.1039/C9NH00209J
[23]
Li M, Gao K, Wan X, et al. Solution-processed organic tandem solar cells with power conversion efficiencies > 12%. Nat Photonics, 2016, 11, 85 doi: 10.1038/nphoton.2016.240
[24]
Meng L, Zhang Y, Wan X, et al. Organic and solution-processed tandem solar cells with 17.3% efficiency. Science, 2018, 361, 1094 doi: 10.1126/science.aat2612
[25]
Cui Y, Yao H, Gao B, et al. Fine-tuned photoactive and interconnection layers for achieving over 13% efficiency in a fullerene-free tandem organic solar cell. J Am Chem Soc, 2017, 139, 7302 doi: 10.1021/jacs.7b01493
[26]
Aqoma H, Imran I F, Wibowo F T A, et al. High-efficiency solution-processed two-terminal hybrid tandem solar cells using spectrally matched inorganic and organic photoactive materials. Adv Energy Mater, 2020, 10, 2001188 doi: 10.1002/aenm.202001188
[27]
Lang K, Guo Q, He Z, et al. High performance tandem solar cells with inorganic perovskite and organic conjugated molecules to realize complementary absorption. J Phys Chem Lett, 2020, 11, 9596 doi: 10.1021/acs.jpclett.0c02794

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    Received: 15 January 2021 Revised: Online: Accepted Manuscript: 15 January 2021Uncorrected proof: 15 January 2021Published: 08 February 2021

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      Article Navigation >  Journal of Semiconductors  > 2021  >  42(2): 020501
      Ling Liu, Zuo Xiao, Chuantian Zuo, Liming Ding. Inorganic perovskite/organic tandem solar cells with efficiency over 20%[J]. Journal of Semiconductors, 2021, 42(2): 020501. doi: 10.1088/1674-4926/42/2/020501 ****L Liu, Z Xiao, C T Zuo, L M Ding, Inorganic perovskite/organic tandem solar cells with efficiency over 20%[J]. J. Semicond., 2021, 42(2): 020501. doi: 10.1088/1674-4926/42/2/020501.
      Citation:
      Ling Liu, Zuo Xiao, Chuantian Zuo, Liming Ding. Inorganic perovskite/organic tandem solar cells with efficiency over 20%[J]. Journal of Semiconductors, 2021, 42(2): 020501. doi: 10.1088/1674-4926/42/2/020501 ****
      L Liu, Z Xiao, C T Zuo, L M Ding, Inorganic perovskite/organic tandem solar cells with efficiency over 20%[J]. J. Semicond., 2021, 42(2): 020501. doi: 10.1088/1674-4926/42/2/020501.
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      Inorganic perovskite/organic tandem solar cells with efficiency over 20%

      doi: 10.1088/1674-4926/42/2/020501
      • 1.

        Center for Excellence in Nanoscience (CAS), Key Laboratory of Nanosystem and Hierarchical Fabrication (CAS), National Center for Nanoscience and Technology, Beijing 100190, China

      • 2.

        University of Chinese Academy of Sciences, Beijing 100049, China

      More Information
      • Ling Liu：got her BS degree from Sichuan Agricultural University in 2017. Now she is a PhD student at University of Chinese Academy of Sciences under the supervision of Professor Liming Ding. She has been working in Liming Ding Lab at National Center for Nanoscience and Technology since 2017. Her research focuses on organic solar cells and perovskite solar cells
      • Zuo Xiao：got his BS and PhD degrees from Peking University under the supervision of Professor Liangbing Gan. He did postdoctoral research in Eiichi Nakamura Lab at the University of Tokyo. In March 2011, he joined Liming Ding Group at National Center for Nanoscience and Technology as an associate professor. In April 2020, he was promoted to be a full professor. His current research focuses on organic solar cells
      • Chuantian Zuo：received his PhD degree in 2018 from National Center for Nanoscience and Technology (CAS) under the supervision of Professor Liming Ding. Then he did postdoctoral research in CSIRO, Australia. Currently, he is an assistant professor in Liming Ding Group. His research focuses on innovative fabrication techniques for perovskite solar cells
      • Liming Ding：got his PhD from University of Science and Technology of China (was a joint student at Changchun Institute of Applied Chemistry, CAS). He started his research on OSCs and PLEDs in Olle Inganäs Lab in 1998. Later on, he worked at National Center for Polymer Research, Wright-Patterson Air Force Base and Argonne National Lab (USA). He joined Konarka as a Senior Scientist in 2008. In 2010, he joined National Center for Nanoscience and Technology as a full professor. His research focuses on functional materials and devices. He is RSC Fellow, the nominator for Xplorer Prize, and the Associate Editors for Science Bulletin and Journal of Semiconductors
      • Corresponding author: zuocht@nanoctr.cn; ding@nanoctr.cn
      • Received Date: 2021-01-15
      • Published Date: 2021-02-10

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